Nitrogen

ammonia, liquid, solution and london

Page: 1 2 3 4 5

Nitroso-nitrogen trioxide

is a greenish solid obtained by passing nitric oxide through liquid oxygen, or by the action of air on solid nitric oxide at the temperature of liquid air. It de composes into nitrogen trioxide and nitric oxide above the tem perature of liquid air (R. L. Hasche, 1925).

Nitrogen Halides.—Nitrogen trichloride, NC1,. Nitrogen does not combine directly with halogens, but compounds may be ob tained indirectly. Nitrogen trichloride was obtained by Dulong (i8i i) by the action of chlorine on ammonium chloride solution. It can also be produced by the electrolysis of concentrated ammo nium chloride solution or by treating ammonia with excess of chlorine. Gattermann showed that the latter reaction takes place in three stages: NH2CH-C12=NHC12+ HC1; The intermediate compound monochloramine, has been isolated and forms colourless crystals melting at —66° C. It is unstable and explosive.

Nitrogen trichloride is a very dangerously explosive, volatile, yellow oil, boiling at 71°C. The vapour has a pungent odour and attacks the eyes and mucous membranes. The liquid explodes on contact with many substances or on exposure to bright light, but its solution in benzene may be safely handled in the dark. It is destroyed by ammonia.

Nitrogen iodide.

Courtois (1812) obtained a black explosive

powder by adding iodine to ammonia solution. This so-called "ni trogen iodine" was proved by Chattaway and Orton (1900) to be really the compound NI,NH, and NI, is not known. When dry the substance explodes violently even when touched with a feather; in some cases the moist substance also explodes. It is an active oxidizing agent, and in all probability first forms hypo iodous acid, HOI, in presence of water. It is decomposed on exposure to light.

BIBLIOGRAPHY.-Roscoe

and Schorlemmer, Treatise on Chemistry, vol. i. ; Abegg, Handbuch der anorganischen Chemie, vol. iii., part 3 (Leipzig, 1907, with bibliography) ; Partington, Inorganic Chemistry.

Technical: Worden,

Technology of Cellulose Esters, vol. i., part 2 (1921) ; Waeser, trans. Fyleman, The Atmospheric Nitrogen Industry (1926) ; Partington and Parker, The Nitrogen Industry (1922) (semi popular, with descriptions of processes and plates) ; Hackspill, L'Azote (1922) (brief, but covers a wide field) ; Maxted, Ammonia and the Nitrides (London, 1922) ; Thorpe, Dictionary of Applied Chemistry, detailed articles (London, 1921-27) ; Report of the Nitrogen Products Committee (London, 1919), with Supplementary Report, 1921 (mainly statistical). (J. R. P.)

Page: 1 2 3 4 5